6:07 PM EDT May 14 2016:

Nirvana – “Return Of The Rat”
From the bootleg
  Outcesticide: In Memory of Kurt Cobain

Last song scrobbled from iTunes at Last.fm

Wipers cover, November 1991

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5:31 PM EDT May 14 2016:

Led Zeppelin – “Bonzo’s Montreux”
From the album Coda
(November 19, 1982)

Last song scrobbled from iTunes at Last.fm

Not sure why this didn’t originally contain "Travellin’ Riverside Blues,” but I do love “Poor Tom”